Publications/Abstracts TPV
Abstracts of TPV Publications
- V. P. Khvostikov, P. Y. Gazaryan, S. V. Sorokina, N. S.
Potapovich, A. V. Malevskaya, R. V. Levin, M. Z. Shvarts, and V. M.
Andreev
"Thermophotovoltaic Cells and modules based on GaSb"
Procs. of 22th European Photovoltaic solar energy conference, Milan, Italy, 2007
Abstract: The solar thermophotovoltaic system is a kind of
thermophotovoltaic (TPV) system where the emitter is powered by the
concentrated sunlight. Narrow bandgap PV cells based on GaSb can be
used in such a system as the efficient TPV converters operating with an
infrared energy source of photons emitted from heated up to 1200-1800
0C solar powered emitters. High efficient thermophotovoltaic cells
based on GaSb and InGaAsSb/GaSb have been developed in this work with
the use of the liquid phase epitaxy, MOCVD growth and zinc diffusion
from the gas phase.
Results of manufacture and development of TPV cells and modules of two
types: flat and cylindrical, also results of their testing in outdoor
and indoor conditions are presented. TPV arrays of the cylindrical type
were tested under irradiation of the different length emitters produced
from W and Ta. Emitters used in the measurements were heated by the
4600x concentrated sunlight obtained with the help of a 60x60 cm2
Fresnel lens. PV cells connected in series intended for the conical
system were fabricated and tested under a flash tester. The cells were
fixed on a plate of BeO ceramics soldered on a copper base. The TPV
array in the conical system of four 1 x 1 cm2 GaSb cells connected in
series under a flash tester have showed the open circuit voltage Voc =
1.77 V and the fill factor FF = 66.4 % with the short circuit
photocurrent Isc = 1 A. The array load characteristics of the
cylindrical system obtained with the use of different length emitters
has been investigated. The TPV array in the cylindrical system of three
1 x 1 cm2 GaSb cells connected in parallel had ISC = 3.5 A, VOC = 0.41
V, FF = 62.4 % and Pmax= 0.88 W with tungsten emitter temperature T =
1400 °C. For effective conversion of low-temperature emitter
radiation, photocells based on InGaAsSb/GaSb has been developed and
manufactured. Band gap energy of photoactive InGaAsSb layers was about
0.6 eV. Voc = 0.43 V and FF = 60 % at Jsc ≈ 7 A/cm2 were obtained
in these cells.
The effect of different diffusion profiles of a p-n junction obtained
by etching the anodic oxidation of a diffused layer on the behaviour of
basic characteristics of GaSb TPV cells: the load characteristic fill
factor, the spectral sensitivity, the open circuit voltage was
investigated in detail at different densities of photocell
illumination. High efficient photocells based on GaSb with reduced
internal losses intended for conversion of radiation from the emitters
heated by the concentrated sunlight have been developed and fabricated
by means of the Zn diffusion technique. The optimum depth of the
initial p-n junction etching has been found allowing to obtain maximal
efficiencies for the cell photocurrent densities of up to 5 A/cm2.
The possibility to obtain GaSb TPV cells by means of a non-traditional
diffusion – from a solid state film diffusant – was studied
as well. Realization of this procedure does not require complicated
equipment, gives a possibility to use sources containing several doping
elements and to obtain low surface charge carrier concentration. The
quality of such diffusion p-n junctions was being estimated by 3.5x3.5
mm2 GaSb cell characteristics. The open circuit voltage reached 0.5 V
and the fill factor – 66 % at the current density of 10 A/cm2
with external quantum yield of 0.82-0.87 at the wavelength range of
800-1600 nm. Quite high parameters of the manufactured cells indicate a
good quality of the diffusion p-n junction obtained by diffusion from a
polymer film.
- L. B. Karlina, M. M. Kulagina, N. H. Timoshina, A. S. Vlasov, and V. M. Andreev
"In0.53Ga0.47As/InP conventional and inverted thermophotovoltaic cells with back surface reflector"
Procs. of the 7th World TPV Conference, Madrid, September 2006, pp. 182-188. ISBN:978-0-7354-0392-5
Abstract: Characteristics of conventional and inverted InGaAs/InP
thermophotovoltaic (TPV) cells with a back surface reflector (BSR)
fabricated on electrically active n-type InP substrates are presented.
Thermophotovoltaic cells based on lattice matched
InP–In0.53Ga0.47As heterostructures were fabricated with the use
of LPE and Zn,P diffusion technologies. In the p-n TPV cells
(conventional type, spectral range 600÷1800 nm) with a frontal
p-InGaAs layer, BSR was made on a n-InP substrate. In the n-p structure
(inverted type, spectral range1000-1800 nm) with a frontal bulk
n-InP-window-substrate, BSR was formed on a p–InGaAs layer.
Antireflection coating (ARC) on the frontal cell surface consists of
ZnS/MgF2 layers.
Results of investigation of sub-bangap photons reflection from InP
substrates with a backside MgF2/Au mirror in the range of
1800÷2000nm are described. The reflection of BSR for InP samples
with the doping level in the range of 1x1017÷6x1018cm-3
evidenced a weak dependence on their thickness and doping level. A
reflection of 86÷90% has been measured for substrates 100μm
thick and 80% for ones 400μm thick with ARC.
Study of sub-bandgap photon reflection of p-InGaAs (Zn,P) layers with
surface concentration of 1÷3x1019cm-3 has been also carried out.
A reflection of 68÷77% for 2€4μm layers with
“hybrid” (ohmic contact plus mirror) back-surface reflector
consisted of deposited Cr/Au layers was measured. It was found, that
p-n and n-p thermophotovoltaic 1x1cm2 cells with identical grid design
reveal similar parameters for up to 1A/cm2 current density (VOC=465mV
and FF=64%) and the 76÷80% reflection of the sub-bandgap photons
for wavelengths longer than 1.86μm.
The developed inverted InGaAs TPV cells have been tested under
illumination of silicon carbide high temperature emitter. The
photocurrent density Jsc=7A/cm2, open circuit voltage Voc=0.476V and
fill factor FF=0.691 have been measured in the inverted (without BSR)
InGaAs cell under SiC emitter heated to the temperature of about
1550°C. Both types of devices can successfully be used as TPV cells
for conversion of radiation in the range of 1500-1900K, with 14-15%
efficience.
- J. L. Plaza, V. Corregidor, J. Olvera, C. Algora, and E. Déguez
"Modification of the electrical properties in pure and doped GaSb by doping with Er and Yb"
Procs. of the 7th World TPV Conference, Madrid, September 2006, pp. 99-106. ISBN:978-0-7354-0392-5
Abstract: n-type Te doped Gallium antimonide, Te-doped-Er codoped
GasSb and and Tedoped- Yb-codoped GaSb single crystals have been grown
by using Liquid Encapsulated Czochralski. Carrier mobility, density and
resistivity along the crystal have been obtained. The axial dopant
composition has also been studied by analysing different wafers by
Induced Coupled Plasma (ICP). From these measurements it is concluded
that codoping with Er and Yb greatly reduces the mobility and increases
the resistivity in both cases compared to simply Te doped GaSb.
Secondary Electron Microscopy (SEM) and Energy Dispersive X-Ray (EDX)
analysis have revealed Sb clustering in Er and Yb codoped Te-doped GaSb
samples. These defects could be the responsible for the reduction of
the carrier mobility and the increment in the resistivity. TPV cells,
with size of 4 mm2have been developed in the Te-doped GaSb sample
showing relatively high performance.
- I. Garcia, I. Rey-Stolle, B. Galiana, and C. Algora
"Analysis of tellurium as n-type dopant in GaInP: doping, diffusion, memory effect and surfactant properties"
Journal of Crystal Growth, vol. 298, pp. 794-799, 2007
Abstract: The use of tellurium as n-type dopant for GaAs and InP
has several advantages, including a high incorporation efficiency, the
very high doping levels achievable and a low diffusion coefficient.
However, its use to dope GaxIn1 xP is not straightforward, since it
shows several problems like a remarkable memory effect and an acute
inertia of the material to become Te-doped, which gives rise to gradual
doping profiles. In this paper, all these phenomena are studied and
quantified using secondary ion mass spectroscopy (SIMS) and
electrochemical CV profiling (ECV) measurements. Concerning the gradual
doping profiles, its origin is linked to the interaction of Te and In
in the gas phase and on the growth surface. A phenomenological
explanation is given for this effect although the exact physical
processes behind remain to be defined.
- W. J. Tobler and W. Durisch
"Plasma-spray coated rare-earth oxides on molybdenum disilicide-High temperature stable emitters for thermophotovoltaics"
Journal of Applied Energy, In press, 2007
Abstract: Selective emitters for thermophotovoltaics consisting of
intermetallic alloy MoSi2 substrate with plasma-spray coated rare-earth
oxides ytterbium oxide Yb2O3, Yb-doped garnet Yb1.5Y1.5Al5O12, and
erbium oxide Er2O3 have been successfully tested till 1650 C. The
emitters are fully operable in an oxygen containing atmosphere, are
highly thermal shock stable, and show good selective emitting
properties. Shielding the high out-of-band emittance of the MoSi2
substrate with 4 lm thick Pt intermediate layer has resulted in reduced
radiation power and emittance of the rare-earth oxide film due to
multiple reflections at the interfaces. The novel technique of vacuum
plasma-spray coated rare-earth oxide films on MoSi2 is a promising way
for the production of effective and high temperature stable selective
thermophotovoltaic emitters.
- W. J. Tobler and W. Durisch
"High Performance selective Er-doped YAG emiiters for thermovotovoltaics"
Journal of Applied Energy, Submitted, 2007
Abstract: Selective emitters for thermophotovoltaics have been
produced by vacuum plasma-spray coating of erbium doped garnet
Er1.5Y1.5Al5O12 and Er2O3 on the intermetallic alloy MoSi2. The
emitters are fully operable in an oxygen-containing10 atmosphere at a
temperature of 1600C, are highly thermal-shock stable, and show good
selective-emitting properties. The film thickness of the rare-earth
oxide was varied between 200 and 600 lm and an optimal thickness for
maximum selectivity was found. Measurements with Si and GaSb photocells
have been performed in order to evaluate the optimal combination
emitter photocell for real thermophotovoltaic systems.
- V. M. Andreev, A. S. Vlasov, V. P. Khvostikov, O. A. Khvostikova, and P. Y. Gazaryan
"Full Scale Solar TPV Generator"
Procs. of 22th European Photovoltaic solar energy conference, Milan, Italy, 2007
Abstract: A solar TPV generator development and characterization is
presented. A cost-effective Fresnel lens based double stage sunlight
concentrator ensuring 4600x concentration ratio is used for outdoor
measurements. For the indoor characterization of the TPV part of the
generator a solar simulator based on a 5kW Xe lamp with an ellipsoidal
mirror is used, and its performance is compared with the real
conditions.
TPV modules based on tungsten emitters and GaSb cells were designed,
fabricated and tested at indoor and outdoor conditions. The performance
of tungsten and MoSi2 emitters under concentrated solar radiation was
investigated.
Emitter temperatures in the range of 1400-2000 K, depending on the
emitter size, were measured under the concentrated sun light. The light
distribution in the module has been characterized with both
concentrated solar radiation and solar simulator. The differences in
the light distribution on the system input appear to bring minor
influence on the TPV module performance.
A continuous progress takes place in improvement of gallium antimonide
PV cells. 1x1 cm GaSb TPV cells were fabricated with the use of the
Zn-diffusion and LPE technologies. Efficiencies of 18-18.8% were
obtained at tungsten emitter (1750-2000 K) radiation. The developed
GaSb PV cells appear to be the most relevant for the use in STPV
systems.
The series connection of PV cells was ensured by the use of various
ceramics. The performance of the cells mounted on BeO2 and Al2O3
ceramics was compared under continuous thermal radiation of a graphite
heater simulating the TPV module conditions. A temperature increase of
a PV cell mounted on a water-cooled base with BeO2 or Al2O3 ceramics by
5-15 degrees correspondingly was estimated from the I-V curve
measurements. This estimation is based on both the I-V measurements
under flash-lamp and dark I-V measurements. This leads to a decrease of
the Voc by 5-20 mV and few percent in FF value, which is affordable.
The whole solar TPV system was examined outdoors. The tungsten
emitters, sealed in quartz bulb, displayed themselves stable under
concentrated sunlight. The power output of 5.5 W was measured with a
full-size 24 cell module and 25x12 mm tungsten emitter under the solar
simulator, providing the same power density, as the Fresnel lens
concentrator. The ways for the system improvement are discussed
- W. Durisch, F. Von Roth, and W. J. Tobler
"Advanced in Gas-Fired Thermophotovoltaic Systems"
Journal of Solar Energy Engineering, vol. 129, pp. 416-422, 2007
Abstract: In a first and completely new approach, a vacuum
plasma-spray coating technique was used to deposit selective emitting
rare-earth oxide films of ytterbia Yb2O3 on porous silicon-infiltrated
silicon carbide foams (Si–SiC). The plasma-spray coating
technique offers a new and promising way to produce selective emitting
coatings on different refractory substrates with complex geometries.
The adhesion and thermal shock stability were tested until a film
thickness of 130 m was achieved; the selective emittance of the oxide
coating has been found to be dependent on the film thickness. The
material combination Si–SiC and Yb2O3, however, needs some major
improvement regarding hightemperature stability and high thermal
cycling loads. In a different approach, the advantage of low emitting
Al2O3 fibers and good thermal matching was combined with Yb2O3 slurry
coating of flexible alumina Al2O3 fiber bundles, formed into a
cylindrical shape.
The thin fiber structure tried to imitate the famous incandescent
mantle emitters of Auer von Welsbach, but with a more rugged structure.
Even though the fibers of the woven emitter were thin, the low thermal
conductivity of Al2O3 led to a distinct reduction of the surface
temperature and emittance, and a shielding effect of the radiation
emanating from the hot inner walls by the cooler outer grid structure
was inevitable. Optical filters consisting of a water film and of
transparent conducting oxides (TCO) have been developed and tested to
protect the photocells against overheating and to reflect
nonconvertible off-band radiation back to the emitter. The water film
led to a significant reduction of the cell temperature and increased
cell performance, whereas with the TCO filters only a reduction of the
cell temperature was observed.
- J. Férnanadez, F. Dimroth, E. Olivia, and A. W. Bett
"Development of Germanium TPV cell technology"
Procs. of 22th European Photovoltaic Solar Energy Conference, Milan, Italy, 2007.
Abstract: The efficiency of Ge TPV cells under high power densities
has been optimized by an adaptation of the cell structure and
processing technology. An adequate front- and back-contact structure
was developed. A fill factor of 71 % has been achieved assuming a
micro-structured tungsten emitter spectrum at 1100 °C with an
incident radiation density of 2.5 W/cm2.
A new back-side of the solar cell was developed which combines an
electrical passivation layer for the Ge cell with a back-side mirror
yielding in a high reflection in the infrared range. This new structure
increases the cell spectral response in the long wavelength range
between 1.6 and 2 μm if the diffusion length is comparable or larger
than the thickness of the base layer. Cells with a doping level in the
range of p=1016 cm-3 show an increase of 10 % in voltage using this
structure. An external reflection between 70 % and 80 % was achieved
for wavelengths below the band gap of Ge, allowing to recycle these
photons by heating the TPV emitter.
- L. B. Karlina, V. V. Evstropov, V. S. Kalinovsky, M. M. Kulagina, N. H. Timoshina, A. S. Vlasov, and V. M. Andreev
"In0.53Ga0.47As/InP Thermophotovoltaic Cells with graded doping in the base"
Procs. of 22th European Photovoltaic solar energy conference, Milan, Italy, 2007
Abstract: Characteristics of inverted In0.53Ga0.47As /InP
thermophotovoltaic (TPV) cells with the uniformly doped base grown on
electrically active n-type InP substrates are presented.
Thermophotovoltaic cells based on lattice matched
InP–In0.53Ga0.47As heterostructures were fabricated with the use
of LPE and Zn,P diffusion from a local source in an open system in the
hydrogen atmosphere.
The TPV cells (spectral range of 1000÷1800nm) with different
base and emitter thicknesses have been investigated. These TPV cells
had doping concentrations up to 2÷4x1019cm-3 for the base layers
and up to 2÷5.1017cm-3 for the emitter layers.
From obtained dark I-V characteristics and photovoltaic characteristics
of the InGaAs/InP TPV cell p-n junctions, the dark resistanceless I-V
characteristic has been determined. Note, that the diffusion component
value determining the potential efficiency of the InGaAs/InP photocell
corresponds to the present-day quality of the best InGaAs TPV cells
fabricated by the MOCVD technique.
Electrical measurements using a flash tester reveal the open circuit
voltage of 0.44÷0.49V, the fill factor of 75÷76% at short
circuit current density of 1÷10A/cm2. The calculated
efficiencies for a TPV cell with uniformly doped base are 16÷17%
for the tungsten emitter temperature of 1800÷2000K.
Thus, the developed technique of Zn diffusion from a local source is a
highly efficient low cost method for manufacture of TPV cells and can
be successfully used in industrial production.
- V.P.Khvostikov, P.Y.Gazaryan, O.A.Khvostikova,
S.V.Sorokina, N.S.Potapovich, A.V.Malevskaya, R.V.Levin, M.Z.Shvarts,
V.M.Andreev
"Narrow band gap TPV converters of radiation from the emitters heated by concentrated sunlight"
Procs. of the 21st European Photovoltaic Solar Energy Conference and Exhibition, Dresden, September 2006
Abstract: In this work, high efficient photovoltaic (PV)
cells
based on gallium antimonide have been developed with the use of the
liquid phase epitaxy (LPE), MOCVD and diffusion from the gas phase
techniques. There are intended for conversion of the thermal radiation
of emitters heated by the sunlight. On the ground of investigation of
the LPE temperature regimes and the tellurium doping during the
process, growth epilayers from various melts, three types of GaSb PV
cells with different structures have been fabricated. The maximum
photoluminescence (PL) intensity corresponding to the interband charge
carrier transitions was observed for epitaxial layers grown by LPE and
by MOCVD.
- L.B.Karlina, A.S.Vlasov, M.M.Kulagina,
N.Kh.Timoshina
"Thermophotovoltaic converters based on In0.53Ga0.47As/InP heterostuctures"
Semiconductors, 40, issue 3, pp. 351-355, 2006
Abstract: For production of highly effective photoconverters
good
semiconductor materials with strictly determined parameters are
required. For thermophotovoltaic (TPV) GaSb cells an homogeneous
Tedopin level in the bulk semiconductor of (2-7)•1017cm-3
is required to produce high efficient PV cells by Zn diffusion process
[1-2]. In this paper we propose to investigate the cell performances
obtained on different GaSb:Te wafers (100) and (221) orientation. Based
on classical I(V) measurements and external quantum efficiency (EQE)
curves, we analyse cell performances in order to improve all
fabrication stages like wafer surface preparation, p-type GaSb emitter
elaboration by Zinc diffusion process, anti reflecting coating
deposition and contact realisation. Most of the technological steps are
described in [3]. Today good performances are obtained on both 3.5 x
3.5 mm² (221) and 10 x 10 mm² (100) GaSb cells. We
obtained
an EQE (Figure 1) between 70-76 % in the 800-1600 nm range for the
first one and 80-88 % in the same spectrum for the second one.
Electrical characterisation give respectively a fill factor (FF)
between 67.8 % down to 65.8% in the 1-5 A/cm² range and 67.5 %
down to 52.5% (Figure 2). The open circuit voltage Voc increase from
0.44 V (1 A/cm²) up to 0.49 V (5 A/cm²) for the small
surface
cell. Post-process information like Zn junction depth and profile
obtained by SIMS analysis will help us to understand deeply the cell
behaviour in order to fabricate large TPV arrays (100 cm²) and
to
test them in real Solar TPV system. It is apparent that improvement of
ingot parameters, wafers and “buffer” layers is of
great
importance for fabrication of future cells.
This work has been partially supported by the European Commission
through the funding of the project FULLSPECTRUM (Ref. N:
SES6-CT-2003-502620).
- V.P. Khvostikov, O.A. Khvostikova, P.Y. Gazaryan,
S.V.
Sorokina, N.S. Potapovich, A.V. Malevskaya, M.Z. Shvarts, N.A.
Kaluzhniy, V.M. Andreev, V.D. Rumyantsev
"Photoconverters for solar TPV systems"
Procs. of the 4th World Conference on Photovoltaic Energy Conversion, Hawaii, May 2006
Abstract: Reflection of infrared radiation from n -InP
substrates
with a rear MgF2 /Au mirror is investigated in the wavelength range
1000–2200 nm. It is found that the reflectance weakly depends
on
substrate thickness and free-carrier concentration in the
(0.1–6)× 1018 cm–3range.
Thermophotovoltaic cells based on the InP/In0.53Ga0.47As
lattice-matched heterostructure of p–n and n–p are
fabricated by liquid-phase epitaxy and Zn and P diffusion from a gas
phase. The characteristics of p–n and n–p
thermophotovoltaic cells with an identical configuration of the
contacts of 1 cm2 area are determined. These characteristics are the
open-circuit voltage U oc = 0.465 V, the filling factor FF = 64% at the
current density of 1 A/cm2, and the reflectance
R= 76 − 80% for wavelengths longer than 1.86μm.
- W. Durisch, J.-C. Mayor, King-hang Lam, J. Close
"Performance and output of a polycrystalline photovoltaic module under actual operating conditions"
Procs. of the 21st European Photovoltaic Solar Energy Conference and Exhibition, Dresden, September 2006
Abstract: Polycrystalline silicon, pc-Si, plays a significant
role
in the world's photovoltaic cell and module production. The market
share of pc-Si modules has increased from 51% in 2001 to about 56% at
present. It is expected that pc-Si modules continue to keep this
position for many more years and that their market share will also grow
in the future. Cell and module efficiencies are increasing steadily and
specific module prices will further decline. Therefore the economic
assessment of modules needs to be updated continuously. For this
purpose the annual module output is required. This in turn implies
knowing the impact of climatic parameters on the efficiency. This work
covers extensive outdoor testing of a pc-Si module from Kyocera
(LA361K51S). All tests were performed at PSI’s Solar Test
Facility. The location of PSI represents a typical site in the Swiss
Midland. The module was fixed on a sun tracker and tested under clear
sky conditions as well as under a cloudy sky. During testing, the
global normal irradiance varied between 24 and 946 W/m2,
the
cell temperature between 1 and 42°C, and the relative air mass
between 1.9 and 7.7. About 600 current/voltage characteristics were
acquired, leading to the efficiency as a function of irradiance, cell
temperature and air mass. The data were used to develop a new
efficiency model to determine the efficiency under all relevant
operating conditions. The model contains six parameters, determined by
applying non-linear fitting techniques. Applying transformation
techniques reported on earlier, measurements and the efficiency model
can be compared and validated in two-dimensional representations, Figs.
1 to 3. Fig. 1 shows excellent efficiency behavior over the whole
irradiance range. The STC efficiency (referred to the active cell area)
was found to be 12.7%, corresponding to an STC modul power of 45.7 W.
An efficiency maximum of 13.3% was found at 419 W/m2. Fig. 2 shows a
linear decrease of the efficiency with temperature. Its temperature
coefficient was found to be –0.0493 abs.-%/°C. Fig. 3
shows the dependence of the efficiency for varying air mass. The
efficiency exhibits a maximum at an air mass of 2.55 and fairly good
red light sensitivity in the late afternoon. Even though the module
tested is fairly old (launched in September 1993), it shows very
attractive behavior in the climate of the Swiss Midland. From recent
testing, it is known that today’s advanced pc-Si modules,
e.g.
Kyocera’s module KC125GHT-2, behave even better, at
remarkably
higher efficiency levels.
- V.M.Andreev, A.S.Vlasov, V.P.Khvostikov,
O.A.Khvostikova, P.Y.Gazaryan, N.A.Sadchikov, V.D.Rumyantsev.
"Solar thermophotovoltaic converter with Fresnel lens and GaSb cells"
Procs. of the 4th World Conference on Photovoltaic Energy Conversion, Hawaii, May 2006
Abstract: Developing of a solar thermophotovoltaic system is
being
reported. Theoretical calculations for system parameters (emitter
aperture absorptance, emitter efficiency, PV cell band gap etc.)
optimization and overall efficiency estimation are presented. The
calculations are mainly oriented to make all the parts of the system
matched to each other: the choice of tungsten emitter dimensions, PV
cell material etc. 20% STPV module efficiency is reachable for GaSb
based receiver with a possible increase to 29% for a tandem PV cell and
advanced technology of STPV module. A cost-effective two-stage
concentrator module based on a primary Fresnel lens and secondary
quartz concave-convex lens have been fabricated. Concentration ratio of
~4000x, necessary for obtaining high efficiency of the
concentratoremitter system, is ensured. Two types of TPV receivers are
tested under outdoor conditions (850 W/m2 average direct sun intensity)
and with the solar simulator set up.
Emitter temperatures in the range of 1400-2000K are registered and GaSb
PV cell short circuit current density up to 5 A/cm2
is observed. BeO ceramics is used for mounting the PV cells allowing
high thermal conductivity and series connection of the cells. High PV
efficiency (19% under tungsten emitter irradiation) is obtained in GaSb
TPV cells.
- V.M.Andreev, A.S.Vlasov, V.P.Khvostikov,
O.A.Khvostikova, P.Y.Gazaryan, N.A.Sadchikov
"Sun powered TPV converters based on GaSb cells"
Procs. of the 21st European Photovoltaic Solar Energy Conference and Exhibition, Dresden, September 2006
Abstract: NO ABSTRACT
- V.D.Rumyantsev, V.P.Khvostikov, O.A.Khvostikova,
P.Y.Gazaryan, N.A.Sadchikov, A.S.Vlasov, E.A.Ionova, V.M.Andreev
"Structural Features of a Solar TPV Systems"
Presented at 6th Conference on Thermophotovoltaic Generation of Electricity, Freiburg, June 2004
Abstract: Developed solar TPV system consists of sunlight
tracker, sunlight concentrator,
absorber of concentrated sunlight, selective emitter of radiation,
internal reflectors of radiation
from the emitter, and PV cells cooled by water or forced air. The
concentration ratio exceeding
8000 suns is ensured by the developed 300W dish mirror with secondary
compound parabolic
concentrator. The emitter is made of tungsten evacuated in a vacuum
bulb. To decrease the
losses of the photons emitted back to outside of TPV system, the area
of the emitter surface
exceeds up to 10 times the absorber aperture area. The developed PV
cells based on Ge and
GaSb have a back-surface mirror, which reflects the sub-bandgap photons
to the emitter
increasing its temperature and overall system efficiency.
(PDF version)
- V.M.Andreev, V.P.Khvostikov, O.A.Khvostikova,
V.D.Rumyantsev, P.Y.Gazarjan, A.S.Vlasov
"Solar Thermophotovoltaic Converters: Efficiency Potentialities"
Presented at 6th Conference on Thermophotovoltaic Generation of Electricity, Freiburg, June 2004
Abstract: Solar thermophotovoltaic efficiency is
theoretically estimated using the following
optimisation parameters: sunlight concentration ratio, absorber/emitter
temperature/efficiency,
photon recirculation efficiency and TPV cell parameters. It has been
found that emitter
temperature exceeding 2000 K, absorber/emitter efficiency of 90% and
TPV systems efficiency
exceeding 30% can be obtained at sunlight concentration ratio exceeding
8·103 suns with using
GaSb cells with back surface reflector and grey-body emitter in vacuum.
Utilization of the
selective emitter allows to increase the efficiency: calculated
efficiency of TPV system with
tungsten emitter increases from 30% to 36%.
(PDF version)
- V.P.Khvostikov, V.D.Rumyantsev, O.A.Khvostikova,
M.Z.Shvarts, P.Y.Gazaryan, S.V.Sorokina, N.A.Kaluzhniy, V.M.Andreev
"Thermophotovoltaic Cells Based on Low-Bandgap Compounds"
Presented at 6th Conference on Thermophotovoltaic Generation of Electricity, Freiburg, June 2004
Abstract: High efficiency TPV GaSb and Ge based cells
fabricated by a non-toxic and inexpensive Zn-diffusion technique have
been developed. GaSb based cells optimised for operation with solar
powered photon emitter allowed increasing the efficiencies up to 27-28%
at black body temperature > 2000 K assuming 90% reflection of
sub-bandgap photons.
Combination of the MOCVD technique or LPE growth and Zn diffusion from
the gas phase allows fabricating Ge photocells on the base of the
GaAs/Ge heterostructures, which are characterized by high photocurrent
and open circuit voltage values. Efficiencies of 13% were obtained in
GaAs/Ge TPV cells under the black-body (1700-2100 K) irradiation
assuming the
achieved 90% reflection of sub-bandgap photons.
(PDF version)
- V.P.Khvostikov, V.D.Rumyantsev, O.A.Khvostikova,
P.Y.Gazaryan, N.A.Kaluzhniy, V.M.Andreev
"TPV CELLS BASED ON Ge, GaSb AND InAs RELATED COMPOUNDS FOR SOLAR POWERED TPV SYSTEMS"
Presented at 19th European PV Solar Energy Conference and Exhibition. 7-11 June 2004, Paris
Abstract: Solar powered TPV systems allow using the
high-temperature (> 2000ºC) vacuum emitters that
insures
promises for their efficiency increase. Theoretical estimations show
that efficiencies exceeding 30% can be achieved
in solar TPV systems characterized by the high efficiency of
sub-bandgap photon recirculation. GaSb based cells
with Zn-diffused emitter were developed. GaSb TPV cell efficiencies of
27-28% can be achieved at black body
temperature > 2000 K assuming 90% reflection of sub-bandgap
photons from the cell to emitter. TPV cells based on
the p-GaAs/p-Ge/n-Ge heterostructure have been fabricated by the MOCVD,
LPE and Zn-diffusion process for TPV
and PV solar applications. InAsSbP/InAs cells were fabricated with the
widened photosensitivity in the infrared range
up to 3.5 µm.
(PDF version)
- V.M.Andreev, V.A.Grilikhes, V.P.Khvostikov,
O.A.Khvostikova, V.D.Rumyantsev, N.A.Sadchikov, M.Z.Shvarts
"Concentrator PV modules and solar cells for TPV systems"
accepted for publication in Solar Energy Materials and Solar cells, 84 (2004) pp. 3-17
Abstract: Concentrator technology is considered as a lower
cost alternative to the ''flat'' solar arrays. For high concentration
ratios (500x and higher) the use of high-efficiency III-V solar cells
is very promising and can provide reduced cell cost contribution to the
cost of an installation. The efficiencies of 25-27% were achieved for
the single-junction AlGaAs/GaAs solar cells under 500-1500 suns,
AM1.5d. These cells are applied in the concentrator modules based on a
concept of the small-aperture refractive concentrators. A modified
structure of the high concentration ''all-glass'' PV modules with III-V
solar cells is proposed. In the ''all-glass'' module design, the
secondary small-aperture smooth surface lenses arranged in an
intermediate composite (glass-silicone) panel be inserted between a
panel of the primary composite Fresnel lens concentrators and a panel
of the solar cells. Such a design allows fabricating the modules of
large total area (up to 0.5x1m2) and improving
environmental protection of the cells. The cells as small as 1.2mm in
designated area diameter operating at very high concentration ratio
(more than 1000x) can be used in the developed solar PV modules. Also,
solar thermophotovoltaics (TPV) is discussed and results of the
narrow-gap GaSb and GaAs/Ge cell development for TPV receivers are
presented.
- V.P.Khvostikov, V.D.Rumyantsev, O.A.Khvostikova,
P.Y.Gazaryan, S.V.Sorokina, M.Z.Shvarts, V.M.Andreev
"Photovoltaic cells for solar powered TPV systems"
31st IEEE PVSC, Coronado Springs Resort, Florida, USA, January 2005
- T.Schlegl, O.V.Sulima, A.W.Bett
"The Influence of Surface Preparation on Zn-Diffusion Processes in GaSb"
accepted for publication in Proceedings of TPV-6, Freiburg, 2004
Abstract: Zinc diffusion is an established process for doping
III-V semiconductors. The experimentally observed kink-and-tail Zn
doping profile in GaSb can be explained by two different diffusion
mechanisms. However, the reproducibility of the doping profile strongly
depends on the treatment of the wafers before the diffusion process.
Significant changes in the doping profile have been observed even under
small variation in surface preparation. It is found that surface oxides
strongly influence Zn profiles. Oxides change the solubility of Zn in
GaSb and appear to influence the diffusion mechanism. Different
cleaning procedures also alter the profile. This can be explained by
defects resulting from cleaning residues. Various surface preparation
methods and their resulting doping profiles are discussed.
- V.P. Khvostikov, O.A.Khvostikova, P.Yu.Gazaryan,
M.Z.Shvarts, V.D.Rumyantsev, V.M.Andreev
"Thermophotovoltaic cells for conversion of thermal radiation and concentrated sunlight to electricity"
Semiconductors, 38, No.8 (2004) pp. 950-955
Abstract: The potential of the thermophotovoltaic conversion
of thermal and solar energy to electricity using narrow-gap
semiconductor photoconverters is shown. Liquid-phase epitaxy,
metal-organic chemical vapor deposition, and Zn diffusion from the
vapor phase are used to fabricate thermophotovoltaic converters based
on GaSb and GaAs/Ge structures and characterized by increased values of
both photocurrent and open-circuit voltage. This circumstance made it
possible to obtain thermophotovoltaic cells that were based on the
aforementioned structures and had efficiencies of 25% (GaSb) and 16%
(GaAs/Ge) at a blackbody-radiation temperature of T = 1473 K under the
condition of 100% return of low-energy photons to the emitter.
- D. Martín and C. Algora
"Temperature-dependent GaSb material parameters for reliable thermophotovoltaic cell modelling"
Semicond. Sci. Technol. 19 (2004) 1040-1052
Abstract: GaSb photovoltaic cells are the most common choice
for receivers in thermophotovoltaic (TPV) systems. Although nowadays
their manufacturing technology is well established, a theoretical
simulation frame for their modelling under real TPV operating
conditions is still not fully developed. This is basically due to the
lack of a reliable and accurate set of GaSb material parameters as
input for the semiconductor simulation tools. Thorough GaSb TPV cell
models are needed to understand the electro-optical behaviour of the
cells and eventually are essential in improving their design. This work
will try to go beyond this key issue, carefully analysing and reviewing
some of the key parameters for GaSb. A complete set of material
parameters, including revised values for the intrinsic concentration,
the electron and hole mobilities and the absorption coefficient, is
given based on extended reviews of previously published data. For the
first time, estimations for their temperature dependences are
introduced. Finally, GaSb TPV cells are manufactured and characterized
inside a real TPV system prototype. The comparisons between the
electrical measurements and the model theoretical predictions confirm
the validity of the proposed set of GaSb material parameters and their
temperature dependences.
- J. Vincent, D. Martín, V.
Bermúdez, C. Algora and E. Diéguez
"GaSb polycrystalline wafers for TPV cell manufacturing"
Proc. of 6th conference on TPV Generation of Electricity
- C. M. Ruiz, O. Vigil, C. Algora, D.
Martín, V. Bermúdez and E. Diéguez
"Transparent conducting oxides as antireflection coating for GaSb TPV cells"
Proc. of 6th conference on TPV Generation of Electricity
- D.Martín and C.Algora
"Theoretical Comparison between GaSb Diffused and Epitaxial TPV Cells"
Proceedings of the 6th International Conference on Thermophotovoltaic Generation of Electricity, 14-16 June 2004, Freiburg, Germany
Abstract: This work deals with the analysis and optimization
of GaSb TPV cells. First, the best configuration for the classical
Zn-diffused structures is discussed, regarding both the semiconductor
structure and grid designs for different illumination conditions. Then,
the theoretical performance of both p/n and n/p GaSb epitaxial cell
structures is calculated and compared to the diffused cell approach,
weighing up the potential benefits of each option.
- V.D.Rumyantsev, V.P.Khvostikov, N.A.Sadchikov,
A.S.Vlasov, V.M.Andreev
"Structural features of a solar TPV system"
Proceedings of the 6th Conference on Thermophotovoltaic Generation of Electricity, Freiburg, 14-16 June 2004
- V.M.Andreev, V.P.Khvostikov, O.Khvostikova,
V.D.Rumyantsev, P.Kazarjan, S.V.Sorokina
"Solar thermophotovoltaic converters"
Accepted at 6th Conference on Thermophotovoltaic Generation of Electricity, Freiburg, 14-16 June 2004
- B.Bitnar, W.Durisch, G.Palfinger, F. von Roth,
U.Vogt, A.Bronstrup, D.Seiler
"Practical thermophotovoltaic generators"
Semiconductors, No.8, 2004, pp. 980-984
Abstract: For use in gas fired thermophotovoltaic systems, a
selective emitter made from Yb2O3
foam ceramic has been developed. This foam ceramic is mechanically
stable and FTIR spectroscopy showed that 10% of the radiation power
emitted by the foam can be converted by Si photocells. The thermal and
thermal-shock stability of Yb2O3
foam ceramic was analysed. The foam passed 200 heating / cooling cycles
without major damage. Tubes were manufactured from this material and
tested in a thermophotovoltaic demonstration system. An electrical
power of 86W was achieved at a thermal power of 16 kW. Using a
simulation model, a potential efficiency of a thermophotovoltaic system
based on our technology applied for the conversion of concentrated
solar radiation was estimated.
- V.M.Andreev, V.P.Khvostikov, O.A.Khvostikova,
P.Y.Gazaryan, N.A.Sadchikov, A.S.Vlasov, V.D.Rumyantsev
"Solar thermophotovoltaic system with high-temperature tungsten emitter"
Accepted for publication in Proceedings of 31st IEEE PVSC, Florida, USA, January 2005
- V.M.Andreev, V.P.Khvostikov
"Solar thermophotovoltaic converters"
Proceedings of the 3rd Workshop "The Path to Ultra-High Efficient Photovoltaics", JRC Ispra, Italy, European Commission, 2004, pp. 83-102
Abstract: The paper presents the review of solar
thermophotovoltaic converters design as well as the growth, material
characterization and device performance of TPV cells based on Ge, Si,
InGaAs/InP and GaSb with related solid solutions. Zinc-diffused
(p-n)-Ge based PV cells were fabricated with short circuit current
density of 33.2 mA/cm2 obtained from the
spectral curve of the internal quantum yield at active area under
sunlight with ë ƒn> 900 nm AM0 spectrum. Ge
cells with GaAs windows were developed by the combination of LPE or
MOCVD growth of GaAs and Zn-diffusion. Efficiency higher than 13% was
obtained in p-GaAs/(p-n)-Ge cells with ƒnunder cut off
ë ƒnƒn> 900 nm AM0 spectrum at
photocurrent densities range of 3-25 A/cm2. The
higher efficiencies have been obtained in TPV cells based on GaSb and
InGaAs (lattice matched to InP substrate): external quantum yield as
high as 90% in IR-part of photosensitivity spectrum; Voc=0.45-0.52 V;
FF=0.7-0.8 at photocurrent densities of 1-5 A/cm2.
A reproducible and low-cost Zn-diffusion technology to n-GaSb wafers
have been developed for producing the high efficiency TPV cells, which
are being used for TPV generators. Significant results for the growth,
material characterization and device performance of TPV cells based on
InGaAsSb, InGaSb, AlGaAsSb, and InAsSbP fabricated by LPE, MOCVD, and
diffusion methods are reviewed. For singlejunction TPV cells, epitaxial
heterostructures with a ~0.53-eV bandgap InGaAsSb base layer and
widebandgap AlGaAsSb or GaSb window/cladding layers (all closely
lattice-matched to a GaSb substrate) represent the state of the art. As
an alternative, a low-cost Zn-diffusion technology for fabrication of
InGaAsSb p-n homojunction structures has been developed for producing
the high efficiency TPV cells. External quantum yields as high as 90%
at wavelengths (around 2000-nm wavelength), and response edges to about
2400 nm wavelength have been obtained with these TPV cells. Another
approach for receiving the perspective TPV devices with bandgaps of
0.55-0.74 eV has been realized by growth of the lattice-matched and
mismatched InGaAs layers on InP substrates. Monolithic interconnected
modules (MIMs) on semi-insulated InP-substrates ensure a decrease of
the Joule losses and an increase of subbandgap photon reflection in the
structures with back-surface reflector that should contribute to TPV
system efficiency owing to photon recirculation.
- Michael Neil Simcock, Jean-Louis Santailler,
Pierre Dusserre, Nathalie Giacometti
"Zinc Diffusion In GaSb For Thermophotovoltaic Cell Applications"
TPV6 Sixth Conference on Thermophotovoltaic Generation of Electricity, June 14-16, 2004, Freiburg Germany
Abstract: Zinc diffusion profiles as a function of depth are
investigated in Te dopes polycrystalline GaSb using SIMS and AFM. Two
types of profile are found; a gradual-profile, which is caused by Zn
deposits on the surface, and a step-profile, which is representative of
the Zn gradient within the GaSb. It is found that the Zn deposits mask
the step-profile to produce the gradual profile. The stepprofile within
the material is different from the so-called "kink and tail" seen in
other studies of the zinc profile within the GaSb. An activation energy
of ~1.1eV is also found, which is lower that in other studies. These
results are discusses in relation to the literature.
